期刊
CHEMICAL SOCIETY REVIEWS
卷 46, 期 3, 页码 603-631出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cs00436a
关键词
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资金
- National Natural Science Foundation of China [51502068]
- Natural Science Foundation of Zhejiang Province [LQ16B030002]
- National Basic Research Program of China [2013CB632404]
- Natural Science Foundation of Zhejiang Province for Distinguished Young Scholars [LR15E020001]
Solar H-2 generation from water has been intensively investigated as a clean method to convert solar energy into hydrogen fuel. During the past few decades, many studies have demonstrated that metal complexes can act as efficient photoactive materials for photocatalytic H-2 production. Here, we review the recent progress in the application of metal-complex chromophores to solar-to-H-2 conversion, including metal-complex photosensitizers and supramolecular photocatalysts. A brief overview of the fundamental principles of photocatalytic H-2 production is given. Then, different metal-complex photosensitizers and supramolecular photocatalysts are introduced in detail, and the most important factors that strictly determine their photocatalytic performance are also discussed. Finally, we illustrate some challenges and opportunities for future research in this promising area.
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