期刊
CHEMICAL COMMUNICATIONS
卷 53, 期 13, 页码 2142-2145出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc10145c
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资金
- National Natural Science Foundation of China (NSFC) [21573103, 21661130149]
- Oppenheimer Foundation (M. A. H.)
- Cambridge Commonwealth Trusts (D. M. H.)
- Royal Society Newton Fund
- EPSRC [EP/L022524/1]
- EPSRC [EP/L022524/1, EP/K005138/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K005138/1, EP/L022524/1] Funding Source: researchfish
Surface-selective direct O-17 DNP has been demonstrated for the first time on CeO2 nanoparticles, for which the first three layers can be distinguished with high selectivity. Polarisation build-up curves show that the polarisation of the (sub-) surface sites builds up faster than the bulk, accounting for the remarkable surface selectivity.
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