期刊
ACS APPLIED MATERIALS & INTERFACES
卷 9, 期 7, 页码 6163-6170出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b14580
关键词
carbon nanotube; Ag nanoparticle; composite; intense pulsed light irradiation; patterning; flexible conductive electrode
资金
- Ministry of Trade, Industry & Energy (MOTIE, Korea) under Advanced Technology Center (ATC) Program [10067668]
- Technology Innovation Program [10052802]
- National Research Foundation of Korea (NRF) - Korean government (MSIP) [2012R1A3A2026417]
- Korea Evaluation Institute of Industrial Technology (KEIT) [10067668] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Recently, highly flexible conductive features have been widely demanded for the development of various electronic applications, such as foldable displays, deformable lighting, disposable sensors, and flexible batteries. Herein, we report for the first time a selective photonic sintering-derived, highly reliable patterning approach for creating extremely flexible carbon nanotube (CNT)/silver nanoparticle (Ag NP) composite electrodes that can tolerate severe bending (20 000 cycles at a bending radius of 1 mm). The incorporation of CNTs into a Ag NP film can enhance not only the mechanical stability of electrodes but also the photonic-sintering efficiency when the composite is irradiated by intense pulsed light (IPL). Composite electrodes were patterned on various plastic substrates by a three-step process comprising coating, selective IPL irradiation, and wiping. A composite film selectively exposed to IPL could not be easily wiped from the substrate, because interfusion induced strong adhesion to the underlying polymer substrate. In contrast, a nonirradiated film adhered weakly to the substrate and was easily removed, enabling highly flexible patterned electrodes. The potential of our flexible electrode patterns was clearly demonstrated by fabricating a light-emitting diode circuit and a flexible transparent heater with unimpaired functionality under bending, rolling, and folding.
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