期刊
FARADAY DISCUSSIONS
卷 199, 期 -, 页码 101-114出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6fd00239k
关键词
-
资金
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]
We developed a special electrochemical cell enabling quantitative analysis and in situ X-ray nanotomography of metal/electrolyte interfaces subject to corrosion. Using this cell and applying the nodoid model to describe menisci formed on tungsten wires during anodization, the evolution of the electrolyte surface tension, the concentration of reaction products, and the meniscus contact angle were studied. In contrast to the electrowetting effect, where the applied electric field decreases the contact angle of electrolytes, anodization of the tungsten wires increases the contact angle of the meniscus. Hence, an electric field favors dewetting rather than wetting of the newly formed surface. The discovered effect opens up new opportunities for the control of wetting phenomena and calls for the revision of existing theories of electrowetting.
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