期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 56, 期 19, 页码 5263-5266出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201701523
关键词
arylation; C-H activation; iodonium compounds; N-heterocycles
资金
- EPSRC
- Marie Curie actions (intra-European fellowship)
- EPSRC [EP/K013599/1] Funding Source: UKRI
- Biotechnology and Biological Sciences Research Council [1595377] Funding Source: researchfish
- Engineering and Physical Sciences Research Council [1237115, EP/K013599/1] Funding Source: researchfish
Both aryl components of diaryliodonium salts can be used in a domino one-pot reaction via in situ generation of a directing group. A number of heterocycles undergo N-arylation which is followed by ruthenium-catalyzed C-arylation. Notably the reaction extends well to unsymmetrical diaryliodonium salts with a number of highly selective examples shown.
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