期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 56, 期 21, 页码 5825-5828出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201702406
关键词
enantioselective catalysis; ester hydrogenation; ferrocene; manganese; reduction
资金
- EPSRC
- Engineering and Physical Sciences Research Council [1398296, 1654521] Funding Source: researchfish
Anew hydrogenation catalyst based onamanganese complex of a chiral P,N,N ligand has been found to be especially active for the hydrogenation of esters down to 0.1 mol% catalyst loading, and gives up to 97% ee in the hydrogenation of pro-chiral deactivated ketones at 30-50 degrees C.
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