期刊
CHEMICAL ENGINEERING & TECHNOLOGY
卷 40, 期 5, 页码 973-980出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ceat.201600594
关键词
Carbon dioxide fixation; Catalyst characterization; Copper; Supported catalysts; Reverse water gas shift
资金
- Sustainable Process Industry through Resources an Energy Efficiency (SPIRE) call under the European Union's Horizon 2020 research and innovation programme [637016]
- Slovenian Research Agency [P2-0152]
- project Direct Conversion of Methane [J2-7319]
Cu-based bifunctional materials were examined for carbon dioxide conversion, thus producing the syngas from hydrogen, which can be attained using surplus electrical energy. Catalysts were synthesized by deposition-precipitation fabrication method, i.e., copper on Al2O3, CeO2, SiO2, TiO2, and ZrO2. To investigate chemical reaction kinetics, the turnover was screened in a parallel high-throughput packed-bed reactor system. The results indicated that catalytic pathway mechanisms were affected by the substrate. An optimal supporting oxide may thus contribute to the engineering and intensification of unconventional feedstock processing, e.g., CO2, as well as the design of emerging catalysis routes. The produced synthesis gas may be readily used for basic chemical platforms, such as methanol.
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