期刊
CHEMCATCHEM
卷 9, 期 10, 页码 1754-1757出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201601627
关键词
AEI zeolites; heterogeneous catalysis; iron zeolites; selective catalytic reduction of NOx; SSZ-39
资金
- Spanish Government-MINECO through the Severo Ochoa [SEV 2012-0267]
- Haldor-Topsoe
- European Union [ERC-AdF-2014-671093]
- Fundacion Ramon Areces
- MINECO [BES-2013-064347]
- [MAT2015-71261-R]
The preparation of the iron-containing SSZ-39 zeolite is described for the first time through two different synthesis methods: post-synthetic cation exchange and one-pot synthesis. The nature and stability of the iron species within the different Fe-SSZ-39 materials have been studied through different characterization techniques, and their catalytic activity has been evaluated for the selective catalytic reduction (SCR) of NOx with ammonia. The directly synthetized Fe-SSZ-39 performs better for the SCR of NOx with ammonia than other related Fezeolites, particularly at elevated reaction temperatures (above 450 degrees C), and presents improved hydrothermal stability when aged under severe conditions.
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