期刊
CHEMISTRY LETTERS
卷 46, 期 6, 页码 780-788出版社
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.161189
关键词
Photoredox system; CO2 fixation; Coenzyme of biocatalyst
资金
- Japan Society for the Promotion of Science [15K14239]
- [2406]
- Grants-in-Aid for Scientific Research [15K14239] Funding Source: KAKEN
In this review, the recent studies on 1) the visible-light-induced reduction of CO2 to formic acid catalyzed by formate dehydrogenase (FDH) via the reduction of a 4,4'- or 2,2'-bipyridinium salt (BP2+) by a photosensitizer, 2) the electrochemical properties of BP2+, and 3) the enzymatic kinetic properties of the interaction between the reduced forms of BP2+ and FDH are reviewed. Moreover, visible-light-induced biocatalytic C-C bond formation using CO2 as a feedstock via photoreduction of the phenylviologen derivative is introduced.
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