期刊
CHEMICAL ENGINEERING JOURNAL
卷 317, 期 -, 页码 821-843出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2017.02.124
关键词
Fly ash; Recycling; Zeolites; Mesoporous materials; Aerogel; Adiabatic foam
资金
- Energy Technology Development Program - Ministry of Trade, Industrial and Energy of the Korean government [20141010101840]
- Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [NRF-2015R1A4A1042434]
- Korea Evaluation Institute of Industrial Technology (KEIT) [20141010101840] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [2015R1A4A1042434] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Large quantities of fly ash are discharged as a by-product from coal power plants. Therefore, an effective method to recycle this waste material is necessary. In this regard, the high silica content of fly ash makes it a potential useful source for the synthesis of nanoporous materials, such as zeolites, mesoporous silica or silica aerogels. In this mini review, zeolite synthesis from fly ash was examined by considering the ash composition, pretreatment procedures, and hydrothermal synthesis conditions (substrate composition and synthesis temperature/time) to identify an optimal set of synthesis conditions. These zeolites can be used as adsorbents and ion-exchangers for environmentally hazardous materials including those present in the fly ash itself. The synthesis of mesoporous silica materials with a high surface area and large pore volume derived from fly ash was next assessed for their use as a support and as a surface-functionalized host for capturing the global warming CO2 and rare earth metal ions. Lastly, the utilization of fly ash for the preparation of silica aerogels or adiabatic foams, which are being considered as a potential building insulation materials, was briefly examined. Cases of synthesizing these nanoporous materials using other solid wastes as silica and/or alumina sources were also examined. The synthesis of diverse porous materials utilizing the waste sources would enable a high level of recycling for a sustainable society with a low environmental burden. (C) 2017 Elsevier B.V. All rights reserved.
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