期刊
ACS NANO
卷 11, 期 6, 页码 5358-5366出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.7b01688
关键词
nanodiamond; superconductivity and ferromagnetism; spin fluctuations; giant positive magnetoresistance; anomalous Hall effect
类别
资金
- Methusalem Funding by the Flemish Government
- KU Leuven Research Fund [GOA/14/007, IDO/11/007, C14/15/053]
- Slovak National Grants [APVV-14-0605, VEGA 1/0409/15, VEGA 2/0149/16]
- U.S. Steel Kosice
- EU ERDF-ITMS [26220120047]
- Helmholtz Association [VH-NG-713]
- UK EPSRC
- Grant Agency of CR [P108-12G-108]
- FWO [G.0962.13, G.0B39.15]
- European Research Council for ERC-Stg LIGHT [307523]
- European Research Council (ERC) [307523] Funding Source: European Research Council (ERC)
Superconductivity and ferromagnetism are two mutually antagonistic states in condensed matter. Research on the interplay between these two competing orderings sheds light not only on the cause of various quantum phenomena in strongly correlated systems but also on the general mechanism of superconductivity. Here we report on the observation of the electronic entanglement between superconducting and ferromagnetic states in hydrogenated boron-doped nanodiamond films, which have a superconducting transition temperature T-c similar to 3 K and a Curie temperature T-Curie > 400 K. In spite of the high T-Curie, our nano-diamond films demonstrate a decrease in the temperature dependence of temperature dependence of resistivity. These anomalous magnetic and electrical transport properties reveal the presence of an intriguing precursor phase, in which spin fluctuations intervene as a result of the interplay between the two antagonistic Furthermore, the observations of high-temperature ferromagnetism, giant positive magnetoresistance, and anomalous Hall effect bring attention to the potential applications of our superconducting ferromagnetic nanodiamond films in magnetoelectronics, spintronics, and magnetic field sensing.
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