期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 23, 期 32, 页码 7626-7641出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201605066
关键词
attachment; confinement; electrocatalysis; immobilization; surface
资金
- Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences
Electrocatalysts are critically important for a secure energy future, as they facilitate the conversion between electrical and chemical energy. Molecular catalysts offer precise control of structure that enables understanding of structure-reactivity relationships, which can be difficult to achieve with heterogeneous catalysts. Molecular electrocatalysts can be immobilized on surfaces by covalent bonds or through non-covalent interactions. Advantages of surface immobilization include the need for less catalyst, avoidance of bimolecular decomposition pathways, and easier determination of catalyst lifetime. This Minireview highlights surface immobilization of molecular electrocatalysts for reduction of O-2, oxidation of H2O, production of H-2, and reduction of CO2.
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