期刊
CHEMICAL SOCIETY REVIEWS
卷 46, 期 11, 页码 3357-3385出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cs00108h
关键词
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资金
- Ryan Fellowship
- Northwestern University International Institute for Nanotechnology
- Department of Defense
- U.S. Army Research Office
- NSERC
- Army Research Office [W911NF-13-1-0229]
- Defense Threat Reduction Agency [HDTRA1-14-1-0014]
Owing to the vast diversity of linkers, nodes, and topologies, metal-organic frameworks can be tailored for specific tasks, such as chemical separations or catalysis. Accordingly, these materials have attracted significant interest for capture and/or detoxification of toxic industrial chemicals and chemical warfare agents. In this paper, we review recent experimental and computational work pertaining to the capture of several industrially-relevant toxic chemicals, including NH3, SO2, NO2, H2S, and some volatile organic compounds, with particular emphasis on the challenging issue of designing materials that selectively adsorb these chemicals in the presence of water. We also examine recent research on the capture and catalytic degradation of chemical warfare agents such as sarin and sulfur mustard using metal-organic frameworks.
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