期刊
BIORESOURCE TECHNOLOGY
卷 234, 期 -, 页码 115-121出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.biortech.2017.03.009
关键词
Biochar; Hydrogen sulfide (H2S) removal; Biogas cleaning; Micro-nutrient; Sulfate-laden waste streams; Anaerobic treatment
资金
- HATCH grant from the College of Tropical Agriculture and Human Resources (CTAHR), University of Hawaii at Manoa (UHM), USA
- Thailand Research Fund (TRF) through the Royal Golden Jubilee Ph.D. Program [PHD/0133/2553]
- Graduate School, Prince of Songkla University, Thailand
- Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior, Ministerio da Educacao (Capes/MEC), Brazil
Removal of hydrogen sulfide (H2S) from biogas was investigated in a biochar column integrated with a bench-scale continuous-stirred tank reactor (CSTR) treating sulfate-laden wastewater. Synthetic wastewater containing sulfate concentrations of 200-2000 mg SO42-/L was used as substrate, and the CSTR was operated at an organic loading rate of 1.5 g chemical oxygen demand (COD)/L.day and a hydraulic retention time (HRT) of 20 days. The biochar was able to remove about 98.0 (+/- 1.2)% of H2S for the ranges of concentrations from 105-1020 ppmv, especially at high moisture content (80-85%). Very high H2S adsorption capacity (up to 273.2 +/- 1.9 mg H2S/g) of biochar is expected to enhance the H2S oxidation into S-0 and sulfate. These findings bring a potentially novel application of sulfur-rich biochar as a source of sulfur, an essential but often deficient micro-nutrient in soils. (C) 2017 Elsevier Ltd. All rights reserved.
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