期刊
PHYSICAL REVIEW B
卷 95, 期 16, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.95.165406
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资金
- National Science Foundation of USA [DMR-1505852, IIA-1430493]
- Office of Integrative Activities [1430519] Funding Source: National Science Foundation
- Office Of The Director [1430519] Funding Source: National Science Foundation
- Office Of The Director
- Office of Integrative Activities [1430493] Funding Source: National Science Foundation
We report observation of strong and anisotropic third-harmonic generation (THG) in monolayer and multilayer ReS2. The third-order nonlinear optical susceptibility of monolayer ReS2, vertical bar chi((3))vertical bar, is on the order of 10(-18) m(2)/V-2, which is about one order of magnitude higher than reported results for hexagonal-lattice transition metal dichalcogenides such as MoS2. A similar magnitude for the third-order nonlinear optical susceptibility was also obtained for a multilayer sample. The intensity of the THG field was found to be dependent on the direction of the incident light polarization for both monolayer and multilayer samples. A point group symmetry analysis shows that such anisotropy is not expected from a perfect 1T lattice and must arise from the distortions in the ReS2 lattice. Our results show that THG measurements can be used to characterize lattice distortions of two-dimensional materials and that lattice distortions are important for the nonlinear optical properties of such materials.
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