期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 359, 期 11, 页码 1942-1946出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201700066
关键词
C-H activation; cobalt; silver; arene trifluoromethylthiolation
资金
- National Natural Science Foundation of China [21472250, 81402794]
- Key Project of Chinese National Programs for Fundamental Research and Development [2016YFA0602900]
- 1000-Youth Talents Plan
- Start-up Grant from Sun Yat-sen University
The direct trifluoromethylthiolation of arenes was realized via (pentamethylcyclopentadienyl) cobalt(III)-catalyzed C(sp(2))-H activation and coupling with AgSCF3 under the assistance of a directing group. The reaction features redox-neutrality, mild conditions, broad substrate scope, and good functional group tolerance. Preliminary mechanistic studies have been conducted.
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