期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 23, 期 35, 页码 8358-8363出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201700742
关键词
encapsulated structure; graphene; metal cyanides; prussian blue; sodium-ion battery; three-dimensional graphene
资金
- Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning [TP2015002]
- National Natural Science Foundation of China [51673042]
- Deanship of Scientific Research at the King Saudi University through International Research Group Project [IRG14-19]
Facile and controllable integration of metal cyanides (MCs) into three-dimensional graphene (3DG) with advantageous structures is of fundamental importance for the development of superior MC-based electrode materials for electrochemical energy storage and catalysis. Here a facile and versatile spatially-confined Ostwald ripening strategy was developed to synthesize a series of 3DG wrapped MC aerogels with different compositions, size, and structure based on the chemical instability of MC in the reaction system. Remarkably, the integration of Prussian blue (PB) into 3DG, with such unique architecture, largely improves the rate performance and long-term cycling stability of PB as a cathode material for sodium ion batteries.
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