期刊
CHEMISTRY-AN ASIAN JOURNAL
卷 12, 期 12, 页码 1309-1313出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201700555
关键词
alkaloids; asymmetric synthesis; -lycorane; total synthesis; zephyranthine
资金
- National Natural Science Foundation of China [21472019]
An asymmetric route to (-)--lycorane and (-)-zephyranthine, and a formal total synthesis of (+)-clivonine were achieved. A pivotal intermediate, which serves as a potent precursor for the divergent syntheses of these natural products, was accessed by a diastereoselective Pd-catalyzed cinnamylation of an N-tert-butanesulfinyl imine.
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