期刊
CATALYSIS SCIENCE & TECHNOLOGY
卷 7, 期 21, 页码 5113-5119出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cy01254c
关键词
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资金
- 973 Program [2014CB845605, 2012CB821705]
- NSFC [21521061, 21331006, 21520102001]
- Strategic Priority Research Program of Chinese Academy of Sciences [XDB20000000]
- Fujian Key Laboratory of Nanomaterials
Herein, hydrogen production from an aqueous medium over a Zr(IV) metal-organic framework (NU-1000) under visible-light irradiation is presented. Photodeposition of CdS nanoparticles onto NU-1000 gives CdS@NU-1000. A ternary composite that hybridizes CdS with reduced graphene oxide (RGO) (different proportions) and NU-1000 was prepared (CdS@NU-1000/RGO). CdS@NU-1000 and CdS@NU-1000/1%RGO exhibit 9.35 and 12.1 times higher photocatalytic activities than commercial CdS under visible light, respectively. More importantly, in sharp contrast with the obvious deterioration in photoactivity of CdS, CdS@NU-1000/1%RGO displayed significantly enhanced photostability. This study clearly demonstrates the advantage of MOF supported CdS nanoparticles for enhancing the photocatalytic H-2 evolution activity with good stability.
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