期刊
NPJ QUANTUM MATERIALS
卷 2, 期 -, 页码 -出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/s41535-017-0048-1
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资金
- Institute for Basic Science (IBS) in Korea [IBS-R009-G1]
- MGML through the program of Czech Research Infrastructures [LM2011025]
- Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4413]
- Ministry of Science & ICT (MSIT), Republic of Korea [IBS-R009-D1-2017-A00] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
A prototypical quasi-2D metallic compound, 1T-TaS2 has been extensively studied due to an intricate interplay between a Mott-insulating ground state and a charge-density-wave order. In the low-temperature phase, 12 out of 13 Ta4+ 5d-electrons form molecular orbitals in hexagonal star-of-David patterns, leaving one 5d-electron with S = 1/2 spin free. This orphan quantum spin with a large spin-orbit interaction is expected to form a highly correlated phase of its own. And it is most likely that they will form some kind of a short-range order out of a strongly spin-orbit coupled Hilbert space. In order to investigate the low-temperature magnetic properties, we performed a series of measurements including neutron scattering and muon experiments. The obtained data clearly indicate the presence of the short-ranged phase and put the upper bound on similar to 0.4 mu B for the size of the magnetic moment, consistent with the orphan-spin scenario.
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