期刊
CHEMICAL PHYSICS LETTERS
卷 683, 期 -, 页码 521-528出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.cplett.2017.05.052
关键词
-
资金
- French Agence Nationale de la Recherche (ANR-HYDRIDES) [ANR-12-BS05-0011-01]
- Rennes Metropole
- Office for Science and Technology of the Embassy of France in the United States
Experimental measurements and theoretical calculations are reported for rotational energy transfer in the Ar-CO system. Experiments were performed in cold uniform supersonic flows of Ar, using an infrared - vacuum ultraviolet double resonance technique to measure absolute state-to-state rate constants and total relaxation cross sections for rotational energy transfer within the (v = 2) vibrational state of CO in collision with Ar at temperatures from 30.5 to 293 K. Close-coupling calculations were also performed using a recent potential energy surface (Sumiyoshi and Endo, 2015). Very good agreement is obtained between measured and calculated values. (C) 2017 Elsevier B.V. All rights reserved.
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