期刊
ADVANCED ENERGY MATERIALS
卷 8, 期 1, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201701475
关键词
amorphous structures; electrocatalysts; electronic effects; metal boride; oxygen evolution
类别
资金
- National Research Foundation (NRF), Prime Minister's Office, Singapore under its Campus for Research Excellence and Technological Enterprise (CREATE) programs
- College of Engineering, Nanyang Technological University [M4081887]
- academic research fund AcRF, Ministry of Education, Singapore [M4020246, ARC10/15]
- Innovation Foundation of Shenzhen Government [JCYJ20160408173202143]
- Joint Fund of Energy Storage of Qingdao [20160012]
- Fundamental Research Funds of Huazhong University of Science and Technology [3004013109, 0118013089]
Cost-effective and efficient oxygen-evolving electrocatalysts are urgently required for energy storage and conversion technologies. In this work, an amorphous trimetallic boride nanocatalyst (Fe-Co-2.3Ni-B) prepared by a simple approach is reported as a highly efficient oxygen evolution reaction electrocatalyst. It exhibits an overpotential () of 274 mV to deliver a geometric current density (j(geo)) of 10 mA cm(-2), a small Tafel slope of 38 mV dec(-1), and excellent long-term durability at a mass loading of 0.3 mg cm(-2). The impressive electrocatalytic performance originates from the unique amorphous multimetal-metalloid complex nanostructure. From application's point of view, this work holds great promise as this process is simple and allows for large-scale production of cheap, yet efficient, material.
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