期刊
ADVANCED ENERGY MATERIALS
卷 7, 期 23, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201700518
关键词
design strategies; electrocatalysts; energy-conversion reactions; metal-organic frameworks
类别
资金
- Australian Research Council (ARC) through the Discovery Project programs [DP140104062, DP160104866, DP170104464]
- National Natural Science Foundation of China [21576202]
The key challenge to developing renewable and clean energy technologies lies in the rational design and synthesis of efficient and earth-abundant catalysts for a wide variety of electrochemical reactions. This review presents materials design strategies for constructing improved electrocatalysts based on MOF precursors/templates, with special emphasis on component manipulation, morphology control, and structure engineering. Guided by these strategies, recently developed MOF-derived materials have exhibited remarkable activity, selectivity, and stability for various energy-conversion processes, manifesting great potential for replacing precious-metal-based catalysts in next-generation energy devices. Existing challenges and opportunities regarding MOF-derived electrocatalysts are also discussed. It is anticipated that by extending current materials design strategies to a wider range of MOF precursors for various energy-related electrocatalytic reactions, significant advances toward achieving highly efficient electrocatalysts can be made.
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