期刊
ADVANCED ENERGY MATERIALS
卷 7, 期 23, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201700912
关键词
characterization methods; interfaces; microstructural control; perovskite solar cells
类别
资金
- Australian Government through the Australian Renewable Energy Agency (ARENA)
- Australian Centre for Advanced Photovoltaics (ACAP)
- ARC Centre of Excellence in Exciton Science (ACEX)
Organic-inorganic hybrid perovskite solar cells form a new type of thin film photovoltaic technology, which has achieved extraordinary improvements in power conversion efficiency in a relatively short time. To further improve the efficiency and stability of the perovskite solar cells, it is critical to understand and control the microstructure of both the functional materials and their interfaces. Much effort has already been made to understand the microstructure of perovskite solar cells and its influence on their performance. This has proved particularly challenging due to the fragile nature of the organic-inorganic perovskites and the consequent potential for generating artefacts through the application of the characterization methods themselves. In this progress report, an overview of some of the more commonly used characterization methods is given, their possible impact on the materials analyses is evaluated, and the latest developments in the understanding of the microstructure of perovskite solar cells are summarized. The heterogenic nature of the individual perovskite grains and the polycrystalline film as a whole is illustrated, the features and properties of the grain boundaries and the effect they can have on solar cell performance are described, and the interface characterization between the layers in the solar cell devices is discussed.
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