期刊
ACS CATALYSIS
卷 8, 期 1, 页码 304-309出版社
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.7b03719
关键词
photoredox catalysis; acylsilanes; acyl radicals; decatungstate salts; acridinium salts
Acyl radicals were smoothly generated from acylsilanes under photoredox-catalyzed conditions. These radicals were formed upon ultraviolet B (UV-B), solar, or visible light irradiation by using decatungstate and acridinium salts as photocatalysts. Acylation of Michael acceptors and a few styrenes resulted in a smooth preparation of unsymmetrical ketones in yields up to 89%.
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