期刊
NATURE COMMUNICATIONS
卷 8, 期 -, 页码 -出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/ncomms15651
关键词
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资金
- Swiss National Science Foundation [200021_138158]
- Swiss National Science Foundation (NCCR-MUST)
- ETH Zurich
- ERC [307270-ATTOSCOPE]
- Swiss Government Excellence Scholarship
- QUEST-Leibniz Research School Hannover
- Swiss National Science Foundation (SNF) [200021_138158] Funding Source: Swiss National Science Foundation (SNF)
Strong-field photoelectron holography and laser-induced electron diffraction (LIED) are two powerful emerging methods for probing the ultrafast dynamics of molecules. However, both of them have remained restricted to static systems and to nuclear dynamics induced by strong-field ionization. Here we extend these promising methods to image purely electronic valence-shell dynamics in molecules using photoelectron holography. In the same experiment, we use LIED and photoelectron holography simultaneously, to observe coupled electronic-rotational dynamics taking place on similar timescales. These results offer perspectives for imaging ultrafast dynamics of molecules on femtosecond to attosecond timescales.
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