4.8 Article

53-attosecond X-ray pulses reach the carbon K-edge

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NATURE COMMUNICATIONS
卷 8, 期 -, 页码 -

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NATURE PUBLISHING GROUP
DOI: 10.1038/s41467-017-00321-0

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资金

  1. DARPA PULSE program, AMRDEC [W31P4Q1310017]
  2. Army Research Office [W911NF-14-1-0383, W911NF-15-1-0336]
  3. Air Force Office of Scientific Research [FA9550-15-1-0037, FA9550-16-1-0149]
  4. National Science Foundation (NSF) [1506345]

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The motion of electrons in the microcosm occurs on a time scale set by the atomic unit of time-24 attoseconds. Attosecond pulses at photon energies corresponding to the fundamental absorption edges of matter, which lie in the soft X-ray regime above 200 eV, permit the probing of electronic excitation, chemical state, and atomic structure. Here we demonstrate a soft X-ray pulse duration of 53 as and single pulse streaking reaching the carbon K-absorption edge (284 eV) by utilizing intense two-cycle driving pulses near 1.8-mu m center wavelength. Such pulses permit studies of electron dynamics in live biological samples and next-generation electronic materials such as diamond.

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