期刊
CHEMICAL PHYSICS LETTERS
卷 684, 期 -, 页码 279-284出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.cplett.2017.07.005
关键词
Adsorption; Dimethyl ether; FER zeolite; Acid site; Periodic model
资金
- National Basic Research Program of China [NKBRSF2013CB834604]
- National Natural Science Foundation of China [21376235]
The adsorption behavior of dimethyl ether (DME) and carbon dioxide (CO) on FER zeolite with different Si/AI ratios and Al positions was calculated. For pure CO or DME gas, the CO adsorption quantity rises near linearly with pressure, while the DME adsorption quantity firstly rises rapidly but then rises much moderately at higher pressure. For the CO-DME gas mixture, both CO and DME adsorption quantity rises rapidly but then rises much moderately at higher pressure. Further investigation reveals that CO and DME molecules are preferentially located in the 6-MR zone of the 8-MR channel. (C) 2017 Elsevier B.V. All rights reserved.
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