期刊
CHEMICAL SCIENCE
卷 8, 期 1, 页码 742-747出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6sc03194c
关键词
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资金
- French National Research Agency (ANR) [ANR-12-BS07-0024-03, ANR-11-LABX-0003-01, ANR-11-LABX-0011]
- Fondation de l'Orangerie for individual Philanthropy
- Agence Nationale de la Recherche (ANR) [ANR-12-BS07-0024] Funding Source: Agence Nationale de la Recherche (ANR)
Copper is currently extensively studied because it provides promising electrodes for carbon dioxide electroreduction. The original combination, reported here, of a nanostructured porous dendritic Cubased material, characterized by electron microcopy (SEM, TEM) and X-ray diffraction methods, and a water/ionic liquid mixture as the solvent, contributing to CO2 solubilization and activation, results in a remarkably efficient (large current densities at low overpotentials), stable and selective (large faradic yields) electrocatalytic system for the conversion of CO2 into formic acid, a product with a variety of uses. These results provide new directions for the further improvement of Cu electrodes.
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