期刊
CHEMICAL SCIENCE
卷 8, 期 4, 页码 3002-3006出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6sc05246k
关键词
-
资金
- National Key Technology Research and Development Program [2015BAK45B01]
An efficient and convenient synthesis of highly functionalized dihydropyrans has been achieved through rhodium(I)-catalysed tandem C(sp(3))-C(sp(3)) bond cleavage and annulation of oxetanols with alkynes. An enantioselective version was enabled using a Binaphine ligand. Excellent site-selectivity and remarkable enantioretention are obtained for 2-substituted oxetanols.
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