期刊
CURRENT APPLIED PHYSICS
卷 17, 期 10, 页码 1335-1340出版社
ELSEVIER
DOI: 10.1016/j.cap.2017.07.005
关键词
Perovskite; Morphology; Methylamine vapor annealing; Large grains; Microwave detected carrier lifetime; Solar cell
资金
- U.S.-India Partnership to Advance Clean Energy-Research (PACE-R) for the Solar Energy Research Institute for India and the United States (SERIIUS) - U.S. Department of Energy (Office of Science) [DE-AC36-08GO28308]
- U.S.-India Partnership to Advance Clean Energy-Research (PACE-R) for the Solar Energy Research Institute for India and the United States (SERIIUS) - U.S. Department of Energy (Office of Basic Energy Sciences) [DE-AC36-08GO28308]
- U.S.-India Partnership to Advance Clean Energy-Research (PACE-R) for the Solar Energy Research Institute for India and the United States (SERIIUS) - U.S. Department of Energy (Energy Efficiency and Renewable Energy, Solar Energy Technology Program) [DE-AC36-08GO28308]
- Government of India, through the Department of Science and Technology [IUSSTF/JCERDC-SERIIUS/2012]
- Department of Science and Technology (DST), Government of India [SB/S3/EECE/0163/2014]
Spin coated perovslcite thin films are known to have an issue of pinholes & poor morphology control which lead to poor device-to-device repeatability, that is an impediment to scale-up. In this work, Methylamine vapor annealing process is demonstrated which consistently leads to high-quality perovskite thin-films with an average grain-size of 10-15 mu m. The improvement in film morphology enables improvement in effective carrier recombination lifetime, from 21 its in as-deposited films to 54 mu s in vapor-annealed films. The annealed films with large-grains are also more stable in ambient conditions. Devices made on annealed perovskite films are very consistent, with a standard deviation of only 0.7%. Methylamine vapor annealing process is a promising method of depositing large-grain CH3NH3PbI3 films with high recombination lifetime and the devices with improved performance. (C) 2017 Elsevier B.V. All rights reserved.
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