期刊
ACS APPLIED MATERIALS & INTERFACES
卷 9, 期 37, 页码 31691-31698出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.7b04624
关键词
titanium oxide; hollow structure; dye-sensitized solar cell; gold nanoparticle; plasmonic-enhanced effect
资金
- National Natural Science Foundation of China [51772249, 51402236, 51472204]
- Research Fund of the State Key Laboratory of Solidification Processing (NWPU), China [123-QZ-2015]
- Key Laboratory of New Ceramic and Fine Processing
- State Key Laboratory of Control and Simulation of Power System and Generation Equipment (Tsinghua University) [KF201607, SKLD17KM02]
- Fundamental Research Funds for the Central Universities [G2017KY0308]
- Program of Introducing Talents of Discipline to Universities [B08040]
Au-decorated TiO2 hollow spheres (Au-THS) have been successfully synthesized via a facile one-pot solvothermal method. The Au-THS hybrid features unique hollow structure with a large specific surface area of 120 m(2) g(-1) and homogeneous decoration of Au nanoparticles, giving rise to enhanced light harvesting and charge generation/separation efficiency. When incorporated into the active layer of dye-sensitized solar cells (DSSCs), an improved power conversion efficiency of 7.3% is obtained, which is increased by 37.7% compared with the controlled P25 DSSC. The underlying mechanism to rationalize the efficiency enhancement can be mainly attributed to the strong synergistic effect of superior light scattering ability of the THS and the plasmonic-enhanced effect rendered by the Au nanoparticles.
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