期刊
CHEMICAL COMMUNICATIONS
卷 53, 期 73, 页码 10204-10207出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc04877g
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资金
- German academic exchange service
- Max Planck Society
Iron-based metal-organic frameworks (MOFs) with varying porosity are converted by pyrolysis into iron/carbon catalysts with predetermined composition and tailored pore structural features for the Fischer-Tropsch synthesis of lower C-2-C-4 olefins. Significantly higher activity arises for catalysts with higher porosity and decreased iron particle size derived from hierarchical MOF xerogel/aerogel precursors as compared to a purely microporous MOF. Post-synthetic functionalization using sodium and sulfur promoters further enhances the catalytic properties.
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