期刊
BIORESOURCE TECHNOLOGY
卷 241, 期 -, 页码 207-213出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.biortech.2017.04.104
关键词
Microwave; Ex-situ catalysis; Co-pyrolysis; HZSM-5; Bio-oil
资金
- National Natural Science Foundation of China [21466022, 21266022]
- International Science & Technology Cooperation Program of China [2015DFA60170-4]
- Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development [Y707sb1001]
- Science and Technology Research Project of Jiangxi Province Education Department [GJJ150213]
- Innovation and Entrepreneurship Development Fund of Thousand talents program Talent [1001-02102082]
Microwave-assisted fast co-pyrolysis of lignin and polypropylene for bio-oil production was conducted using the ex-situ catalysis technology. Effects of catalytic temperature, feedstock/catalyst ratio, and lignin/polypropylene ratio on product distribution and chemical components of bio-oil were investigated. The catalytic temperature of 250 degrees C was the most conducive to bio-oil production in terms of the yield. The bio-oil yield decreased with the addition of catalyst during ex-situ catalytic co-pyrolysis. When the feedstock/catalyst ratio was 2: 1, the minimum char and coke values were 21.22% and 1.54%, respectively. The proportion of cycloalkanes decreased and the aromatics increased with the increasing catalyst loading. A positive synergistic effect was observed between lignin and polypropylene. The char yield dramatically deceased and the bio-oil yield improved during co-pyrolysis compared with those during lignin pyrolysis alone. The proportion of oxygenates dramatically and the minimum value of 6.74% was obtained when the lignin/polypropylene ratio was 1:1. (C) 2017 Published by Elsevier Ltd.
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