期刊
ACS APPLIED MATERIALS & INTERFACES
卷 9, 期 47, 页码 41104-41110出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.7b12046
关键词
lead sulfide; quantum dots; sensitized solar cells; perovskite; passivation
资金
- National Research Foundation of Korea (NRF) under Ministry of Science, ICT & Future Planning [2014R1A5A1009799, 2017M3A7B4041696, 2009-0093826]
- Kyung Hee University [KHU-20141582]
High-performance solid-state PbS quantum dot-sensitized solar cells (QD-SSCs) with stable 9.2% power conversion efficiency at 1 Sun condition are demonstrated by introduction of hybrid perovskite interlayer. The PbS QDs formed on mesoscopic TiO2 (mp-TiO2) by spin-assisted successive precipitation and anionic exchange reaction method do not exhibit PbSO4 but have PbSO3 oxidation species. By introducing perovskite interlayer in between mp-TiO2/PbS QDs and poly-3-hexylthiophene, the PbSO3 oxidation species are fully removed in the PbS QDs and thereby the efficiency of PbS QD-SSCs is enhanced over 90% compared to the pristine PbS QD-SSCs.
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