期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 56, 期 49, 页码 15658-15662出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201709738
关键词
functionalization; metal-organic frameworks; modular growth; nanostructures; synthesis design
资金
- Fundamental Research Funds for the Central Universities
- program for Young Excellent Talents in Tongji University [2014KJ007]
- Foundation of State Key Laboratory of Pollution Control and Resource Reuse (Tongji University) [PCRRY15007]
- National Natural Science Foundation of China [21501135, 21777119]
- Science & Technology Commission of Shanghai Municipality [17230711600]
- JST
- JSPS KAKENHI [25000007]
- World Premier International Research Initiative (WPI) of MEXT
- Shanghai Tongji Gao Tingyao Environmental Science and Technology Development Foundation (STGEF)
- Grants-in-Aid for Scientific Research [25000007] Funding Source: KAKEN
Fabrication of hybrid MOF-on-MOF heteroarchitectures can create novel and multifunctional platforms to achieve desired properties. However, only MOFs with similar crystallographic parameters can be hybridized by the classical epitaxial growth method (EGM), which largely suppressed its applications. A general strategy, called internal extended growth method (IEGM), is demonstrated for the feasible assembly of MOFs with distinct crystallographic parameters in an MOF matrix. Various MOFs with diverse functions could be introduced in a modular MOF matrix to form 3D core-satellite pluralistic hybrid system. The number of different MOF crystals interspersed could be varied on demand. More importantly, the different MOF crystals distributed in individual domains could be used to further incorporate functional units or enhance target functions.
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