期刊
PHYSICAL REVIEW B
卷 96, 期 22, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.96.224513
关键词
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资金
- National Key Research and Development Program of China [2017YFA0302900, 2016YFA0300300, 2017YFA0303103]
- NSF of China [91321207, 11427805, U1532267, 11604376]
- Strategic Priority Research Program (B) of the Chinese Academy of Sciences [XDB07020300]
- Gordon and Betty Moore Foundation EPiQS initiative [GBMF-4412]
Here we report the in situ high-pressure (up to similar to 50-GPa) Hall-effect measurements on single-crystal black phosphorus. We find a strong correlation between the sign of the Hall coefficient, an indicator of the dominant carrier type, and the superconducting transition temperature (T-C). Importantly, we find a change from electron-dominant to hole-dominant carriers in the simple cubic phase of phosphorus at a pressure of similar to 17.2GPa, providing an explanation for the puzzling valley it displays in its superconducting T-C vs pressure phase diagram. Our results reveal that hole carriers play an important role in developing superconductivity in elemental phosphorus and the valley in T-C at 18.8 GPa is associated with a Lifshitz transition.
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