期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 23, 期 69, 页码 17454-17457出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201704155
关键词
annulation; cobalt(III); heterocycles; internal oxidant; isoquinolone
资金
- SERB [EMR2016/000136]
- IITK
- CSIR
Cp*Co-III-catalyzed highly regioselective mono- and bis-annulation of arylamides with 1,3-diynes using N-OMe as an internal oxidant is demonstrated. This atom-economical transformation does not require any external oxidant and tolerates many functional groups. Various symmetrical and unsymmetrical heterocycles (homo and hetero) are accessed with predictable regio- and chemoselectivity.
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