期刊
SYNLETT
卷 28, 期 7, 页码 835-840出版社
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0036-1588930
关键词
aromatic aldehydes; aryl iodides; reductive carbonylation; ligandless; ambient conditions
资金
- Natural Science Foundation of Jiangsu Province [BK20161553]
- Natural Science Foundation of China [21302099]
- Natural Science Foundation of Jiangsu Provincial Colleges and Universities [16KJB150019]
- SRF for ROCS, SEM
- Qing Lan project
- Priority Academic Program Development of Jiangsu Higher Education Institutions
Ligandless palladium-catalyzed reductive carbonylation of aryl iodides for the synthesis of aromatic aldehydes has been developed. This carbonylation process proceeded effectively even under ambient temperature and pressure. In addition, this method enables successive reductive carbonylation of diiodobenzenes to furnish dialdehydes in satisfactory yields. Finally, the nature of the active catalytic species is discussed.
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