期刊
SOFT MATTER
卷 13, 期 37, 页码 6639-6646出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7sm01456b
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资金
- Fonds de recherche du Quebec - Nature et technologies
- Canada Foundation for Innovation
Diazonium chemistry concomitant with in situ electrochemical reduction was used to graft an aryl aldehyde to indium-tin oxide (ITO) coated glass substrates. This served as an anchor for preparing electroactive azomethines that were covalently bonded to the transparent electrode. The immobilized azomethines could undergo multiple step-wise component exchanges with different arylamines. The write-erase-write sequences were electrochemically confirmed. The azomethines could also be reversibly hydrolyzed. This was exploited for multiple azomethine-hydrolysis cycles resulting in discrete electroactive immobilized azomethines. The erase-rewrite sequences were also electrochemically confirmed.
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