期刊
SCIENCE OF THE TOTAL ENVIRONMENT
卷 609, 期 -, 页码 807-814出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.scitotenv.2017.07.194
关键词
Flocculation; Fractal dimension; Shear rate; Aggregates
资金
- Sao Paulo Research Foundation (Fundacao de Amparo a Pesquisa do Estado de Sao Paulo-FAPESP) [2010/50694-0, 2013/25641-9, 2013/21355-1, 2013/01634-3]
- Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP) [13/25641-9, 13/01634-3, 10/50694-0] Funding Source: FAPESP
The two-dimensional fractal dimension (D-f) of large aggregates of kaolin (>540 mu m) during the shear flocculation process for kaolin solution was investigated using non-intrusive in situ image-based acquisition system. Separate experiments were also carried out for three different sized sub-ranges of large aggregates (0.540-1.125 mm; 1.125-1.750 mm; 1.750-2.375 mm). Digital images were taken at a frequency of 10 Hz for 10 s for each different pairs of gradients of velocity (G(f)) of 20 and 60 s(-1) and flocculation times of 2; 3; 4; 5; 10; 20; 30; 60; 120 and 180 min. For the same conditions, particle size distribution (PSD) was also determined. Under the investigated conditions, the lowest G(f) produced the greatest D-f (1.69) at a flocculation time of 30 min for the whole range of aggregates. Also, the evolution of the longest length of aggregate (l) and D-f with time, showed that the dynamic steady-state was reached at different times for each shear rate and l ranges. However, D-f varied for each size sub-range (ca. 1.1 to 1.8). Finally, the behavior of the aggregate structure may be understood by the predominance of different aggregation mechanisms such as cluster-cluster for G(f) of 60 s(-1) and particle-cluster for G(f) of 20 s(-1). (C) 2017 Elsevier B.V. All rights reserved.
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