期刊
SCIENCE OF THE TOTAL ENVIRONMENT
卷 581, 期 -, 页码 541-549出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.scitotenv.2016.12.162
关键词
Pu isotopes; Soil particles; Size distribution; Wet-sieving; (239+24)pu/(137)cs activity ratio
资金
- National Natural Science Foundation of China [41501286, 41271289, 41671466]
- Natural Science Foundation of Jiangsu Province [BK20150578]
- Fundamental Research Funds for the Central Universities [020914380010, 020914380001]
- National Key R&D Program of China [2016YFA0600502]
Information on how plutonium (Pu) isotopes associate with natural soil particles of different size is very important for the interpretation involved in the application of Pu isotopes as soil erosion tracers. This work investigated the association of Pu isotopes with different particle size fractions of natural soils and compared it with that of Cs-137. Ten bulk soils collected from two different areas were separated into different particle size fractions by a combination of wet sieving and centrifugation techniques and the sub-samples were analyzed for Cs-137, Pu-239 and Pu-240. Results showed that the concentrations of both (239+24) Pu and Cs-137 increase with decreased particle sizes and are closely related to the specific surface areas of soil particles, which demonstrated a similar preferential association of Pu with finer soil particles as Cs-137. The activity ratios of Pu239+24/(CS)-C-137 in soil fractions increasing with increased particle size further indicated a less preferential transport of Pu with fine particles compared to Cs-137. These results not only highlight the suitability of Pu isotopes as soil erosion tracers, but also provide useful information for assessing the migration behavior of Pu in contaminated environments.
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