期刊
CHEMSUSCHEM
卷 11, 期 1, 页码 71-85出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201701590
关键词
biofuels; heterogeneous catalysis; homogeneous catalysis; reaction mechanisms; structure-activity relationships
资金
- National Natural Science Foundation of China (NSFC) [21303163]
- Zhejiang Provincial Natural Science Foundation of China [LY17B060006]
- Xinmiao Talent Program in Zhejiang Province [G1712101057901]
Because n-butanol as a fuel additive has more advantageous physicochemical properties than those of ethanol, ethanol valorization to n-butanol through homo- or heterogeneous catalysis has received much attention in recent decades in both scientific and industrial fields. Recent progress in catalyst development for upgrading ethanol to n-butanol, which involves homogeneous catalysts, such as iridium and ruthenium complexes, and heterogeneous catalysts, including metal oxides, hydroxyapatite (HAP), and, in particular, supported metal catalysts, is reviewed herein. The structure-activity relationships of catalysts and underlying reaction mechanisms are critically examined, and future research directions on the design and improvement of catalysts are also proposed.
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