4.8 Article

Transferability and Generalizability of Regression Models of Ultrafine Particles in Urban Neighborhoods in the Boston Area

期刊

ENVIRONMENTAL SCIENCE & TECHNOLOGY
卷 49, 期 10, 页码 6051-6060

出版社

AMER CHEMICAL SOC
DOI: 10.1021/es5061676

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资金

  1. NIEHS [ES015462, T32 ES198543]
  2. Jonathan M. Tisch College of Citizenship and Public Service (through the Tufts Community Research Center)
  3. U.S. EPA [FP-917203]
  4. P.E.O. Scholar award

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Land use regression (LUR) models have been used to assess air pollutant exposure, but limited evidence exists on whether location-specific LUR models are applicable to other locations (transferability) or general models are applicable to smaller areas (generalizability). We tested transferability and generalizability of spatial-temporal LUR models of hourly particle number concentration (PNC) for Boston-area (MA, U.S.A.) urban neighborhoods near Interstate 93. Four neighborhood-specific regression models and one Boston-area model were developed from mobile monitoring measurements (34-46 days/neighborhood over one year each). Transferability was tested by applying each neighborhood-specific model to the other neighborhoods; generalizability was tested by applying the Boston-area model to each neighborhood. Both the transferability and generalizability of models were tested with and without neighborhood-specific calibration. Important PNC predictors (adjusted-R-2 = 0.24-0.43) included wind speed and direction, temperature, highway traffic volume, and distance from the highway edge. Direct model transferability was poor (R-2 < 0.17). Locally-calibrated transferred models (R-2 = 0.19-0.40) and the Boston-area model (adjusted-R-2 = 0.26, range: 0.13-0.30) performed similarly to neighborhood- specific models; however, some coefficients of locally calibrated transferred models were uninterpretable. Our results show that transferability of neighborhood-specific LUR models of hourly PNC was limited, but that a general model performed acceptably in multiple areas when calibrated with local data.

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