期刊
RADIATION PHYSICS AND CHEMISTRY
卷 135, 期 -, 页码 45-48出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.radphyschem.2017.02.056
关键词
Synchrotron; Rare gas; Mixed clusters; Geometric structure; Co-expansion
资金
- Swedish Research Council (VR)
- Goran Gustafsson Foundation
- Knut and Alice Wallenberg Foundation
- Foundation for International Cooperation in Research and Higher Education (STINT)
- Foundation for Strategic Research
Binary rare gas clusters; xenon and neon which have a significant contrariety between sizes, produced by a co-expansion set up and have been studied using synchrotron radiation based x-ray photoelectron spectroscopy. Concentration ratios of the heterogeneous clusters; 1%, 3%, 5% and 10% were controlled. The core level spectra were used to determine structure of the mixed cluster and analyzed by considering screening mechanisms. Furthermore, electron binding energy shift calculations demonstrated cluster aggregation models which may occur in such process. The results showed that in the case of low mixing ratios of 3% and 5% of xenon in neon, the geometric structures exhibit xenon in the center and xenon/neon interfaced in the outer shells. However, neon cluster vanished when the concentration of xenon was increased to 10%.
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