4.8 Article

Does a Growing Static Length Scale Control the Glass Transition?

期刊

PHYSICAL REVIEW LETTERS
卷 119, 期 19, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.119.195501

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资金

  1. Swiss National Science Foundation [200021-165509]
  2. Simons Foundation [454953]
  3. Royal Society
  4. Swiss National Science Foundation (SNF) [200021_165509] Funding Source: Swiss National Science Foundation (SNF)

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Several theories of the glass transition propose that the structural relaxation time tau(alpha) is controlled by a growing static length scale. that is determined by the free energy landscape but not by the local dynamic rules governing its exploration. We argue, based on recent simulations using particle-radius-swap dynamics, that only a modest factor in the increase in ta on approach to the glass transition may stem from the growth of a static length, with a vastly larger contribution attributable, instead, to a slowdown of local dynamics. This reinforces arguments that we base on the observed strong coupling of particle diffusion and density fluctuations in real glasses.

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