期刊
ACS OMEGA
卷 3, 期 8, 页码 8733-8744出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsomega.8b01234
关键词
-
资金
- Ministry of Science and Technology, Taiwan [MOST 106-2112-M-007016-MY3, MOST 105-3113-E-006-019-CC2]
Carbon nanotube supported ternary metallic nanocatalysts (NCs) comprising Ni-core -Pd-shell structure and Pt atomic scale clusters in shell (namely, Ni@Pd/Pt) are synthesized by using wet chemical reduction method with reaction time control. Effects of Pt4+ adsorption time and Pt/Pd composition ratios on atomic structure with respect to electrochemical performances of experimental NCs are systematically investigated. By cross-referencing results of high-resolution transmission electron microscopy, X-ray diffraction, X-ray absorption, density functional theoretical calculations, and electrochemical analysis, we demonstrate that oxygen reduction reaction (ORR) activity is dominated
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