期刊
ORGANIC LETTERS
卷 19, 期 20, 页码 5557-5560出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b02660
关键词
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资金
- JSPS KAKENHI [JP16H01019, JP16H04109, JP16H06887]
- JST ACT-C, Japan [JPMJCR12ZE]
- Japan Association for Chemical Innovation
- Naito Foundation
- Tokuyama Science Foundation
- Grants-in-Aid for Scientific Research [16H01019, 16H06887] Funding Source: KAKEN
A new class of aromatic metamorphosis in which benzofurans are converted into diverse six-membered oxaheterocycles has been developed. This transformation is composed of two reactions in one pot: manganese-catalyzed arylative or alkylative ring-opening of benzofurans affording dianionic intermediates and subsequent trapping with multivalent heteroatom electrophiles. Various electrophiles containing silicon, boron, phosphorus, germanium, and titanium could be applied to this heteroatom insertion.
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