期刊
ORGANIC LETTERS
卷 20, 期 1, 页码 212-215出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03561
关键词
-
资金
- Natural Science Foundation of China [21472039, 21625203, 21402046]
A novel tandem annulation of N-(o-ethynylaryl)acrylamides, with CH2Cl2 as a one-carbon unit, for the divergent synthesis of cyclopenta[c]quinolin-4(5H)-ones and benzo[j]phenanthridin-6(5H)-ones, which relies on the substitution effect of the 2 position of the acrylamide moiety, is described. Promoted by the visible-light photoredox catalysis, this reaction allows the formation of multiple chemical bonds through multiple C-Cl/C-H functionalizaiion and [2 + 2 + 1] annulation cascades.
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