期刊
ORGANIC LETTERS
卷 19, 期 4, 页码 754-757出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b03546
关键词
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资金
- NSFC [21232004, 21472071, 21602087]
- PAPD of Jiangsu Higher Education Institutions
- Outstanding Youth Fund of JSNU [YQ2015003]
- NSF of Jiangsu Province [BK20151163, BK20160212]
- Qing Lan Project
- NSF of Jiangsu Education Committee [15KJB150006]
Silver-mediated C(sp(3))-H functionalization and 6-endo-dig oxo-cyclization of conjugated beta-alkynyl ketones have been established under oxidative conditions. The reaction leads to the concise formation of a wide range of isochromenes via C(sp(3))-H bond-breaking and radical addition steps. Dual and monofunctional isochromene products were selectively controlled by using either electron-rich or electron-deficient radical sources.
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